A team of physicists from the Paul-Drude-Institut für Festkörperelektronik (PDI) in Berlin, Germany, NTT Basic Research Laboratories in Atsugi, Japan, and the U.S. Naval Research Laboratory (NRL) has used a scanning tunneling microscope to create quantum dots with identical, deterministic sizes. The perfect reproducibility of these dots opens the door to quantum dot architectures completely free of uncontrolled variations, an important goal for technologies from nanophotonics to quantum information processing as well as for fundamental studies. The complete findings are published in the July 2014 issue of the journal Nature Nanotechnology.
Quantum dots are often regarded as artificial atoms because, like real atoms, they confine their electrons to quantized states with discrete energies. But the analogy breaks down quickly, because while real atoms are identical, quantum dots usually comprise hundreds or thousands of atoms - with unavoidable variations in their size and shape and, consequently, in their properties and behavior. External electrostatic gates can be used to reduce these variations. But the more ambitious goal of creating quantum dots with intrinsically perfect fidelity by completely eliminating statistical variations in their size, shape, and arrangement has long remained elusive.
Creating atomically precise quantum dots requires every atom to be placed in a precisely specified location without error. The team assembled the dots atom-by-atom, using a scanning tunneling microscope (STM), and relied on an atomically precise surface template to define a lattice of allowed atom positions. The template was the surface of an InAs crystal, which has a regular pattern of indium vacancies and a low concentration of native indium adatoms adsorbed above the vacancy sites. The adatoms are ionized +1 donors and can be moved with the STM tip by vertical atom manipulation. The team assembled quantum dots consisting of linear chains of N = 6 to 25 indium atoms; the example shown here is a chain of 22 atoms.
Stefan Fölsch, a physicist at the PDI who led the team, explained that "the ionized indium adatoms form a quantum dot by creating an electrostatic well that confines electrons normally associated with a surface state of the InAs crystal. The quantized states can then be probed and mapped by scanning tunneling spectroscopy measurements of the differential conductance." These spectra show a series of resonances labeled by the principal quantum number n. Spatial maps reveal the wave functions of these quantized states, which have n lobes and n - 1 nodes along the chain, exactly as expected for a quantum-mechanical electron in a box. For the 22-atom chain example, the states up to n = 6 are shown.
For nearly a century, “reality” has been a murky concept. The laws of quantum physics seem to suggest that particles spend much of their time in a ghostly state, lacking even basic properties such as a definite location and instead existing everywhere and nowhere at once. Only when a particle is measured does it suddenly materialize, appearing to pick its position as if by a roll of the dice.
This idea that nature is inherently probabilistic — that particles have no hard properties, only likelihoods, until they are observed — is directly implied by the standard equations of quantum mechanics. But now a set of surprising experiments with fluids has revived old skepticism about that worldview. The bizarre results are fueling interest in an almost forgotten version of quantum mechanics, one that never gave up the idea of a single, concrete reality.
The experiments involve an oil droplet that bounces along the surface of a liquid. The droplet gently sloshes the liquid with every bounce. At the same time, ripples from past bounces affect its course. The droplet’s interaction with its own ripples, which form what’s known as a pilot wave, causes it to exhibit behaviors previously thought to be peculiar to elementary particles — including behaviors seen as evidence that these particles are spread through space like waves, without any specific location, until they are measured.
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